These are my favorites, in order.
1. Doctor Octopus...Alfred Molina
2. Loki...Tom Hiddleston
3. Red Skull...Hugo Weaving
4. Magneto...Ian McKellan
5. Mystique...Rebecca Romjin
6. Green Goblin...Willem Dafoe
7. Ultron...James Spader
8. Whiplash...Mickey Rourke
9. Mephisto...Peter Fonda
10. Jigsaw...Dominic West
1. Doctor Octopus...Alfred Molina
2. Loki...Tom Hiddleston
3. Red Skull...Hugo Weaving
4. Magneto...Ian McKellan
5. Mystique...Rebecca Romjin
6. Green Goblin...Willem Dafoe
7. Ultron...James Spader
8. Whiplash...Mickey Rourke
9. Mephisto...Peter Fonda
10. Jigsaw...Dominic West
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