Just discovered these. Many recorded in connection with the 1966 Batman TV series. Some good-some not so good:

Burgess Meredith as the Penguin:

The Escape

http://www.youtube.com/watch?v=1-fQzO7AsIc

The Capture:

http://www.youtube.com/watch?v=H1vUsFrePyE

Frank Gorshin's The Riddler, (composed by Mel Torme`)

http://www.youtube.com/watch?v=EAlfr7wsqcM

Burt Ward, Boy Wonder, I Love You, (by Burt Ward & Frank Zappa):

http://www.youtube.com/watch?v=AjoLQbJCPTI

Adam West, Miranda, (Burt Ward appears):

http://www.youtube.com/watch?v=zZljPX5DSD8